Файл: Doicu A., Wriedt T., Eremin Y.A. Light scattering by systems of particles (OS 124, Springer, 2006.pdf

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134 2 Null-Field Method

gradient methods and iterative approaches [74, 95, 198, 244, 271]. Originally all methods were implemented for spherical particles, but Xu [274] recently extended his computer code for axisymmetric particles.

In the following analysis, we derive (2.144) and (2.145) by using the superposition T -matrix method. The field exciting the lth particle can be expressed as

N

Eexc,l (rl) = Ee (rl) + Es,p (rl) ,

p=l

where Ee is the incident field and Es,p is the field scattered by the pth particle. In the null-field method, transformation rules between the expansion coe cients of the incident and scattered fields in di erent coordinate systems have been derived by using the integral representations for the expansion co- e cients. In the superposition T -matrix method, these transformations are obtained by using the series representations for the electromagnetic fields in di erent coordinate systems. For the external excitation, we consider the vector spherical wave expansion

Ee(r) = aµM 1µ (ksr) + bµN 1µ (ksr)

µ

and use the addition theorem

M µ1 (ksr) =

11 (ksr0l) M ν1 (ksrl) ,

N µ1 (ksr)

Tµν

N ν1 (ksrl)

to obtain

 

 

 

Ee (rl) = al,ν M ν1 (ksrl) + bl,ν N ν1 (ksrl)

ν

 

 

 

with

 

 

 

al,ν =

 

11

(ksr0l) aµ .

bl,ν

 

Tµν

bµ

Similarly, for the field scattered by the pth particle, we consider the series representation

Es,p (rp) = fp,µM 3µ (ksrp) + gp,µN 3µ (ksrp)

µ

and use the addition theorem

M 3µ (ksrp) N 3µ (ksrp)

=

31

(ksrpl) M ν1 (ksrl)

for rl < rpl ,

 

Tµν

N ν1 (ksrl)

 


2.6 Multiple Particles

135

to derive

Es,p (rl) = flp,ν M 1ν (ksrl) + glp,ν N 1ν (ksrl)

ν

with

flp,ν =

31

(ksrpl) fp,µ .

glp,ν

Tµν

gp,µ

Thus, the field exciting the lth particle can be expressed in terms of regular vector spherical wave functions centered at the origin Ol

Eexc,l (rl) = al,ν M ν1

(ksrl) + bl,ν N ν1 (ksrl) ,

ν

 

 

where the expansion coe cients are given by

 

 

 

 

 

 

N

 

 

 

 

[(el)

 

] =

11

(ksr0l)

[eµ] +

 

31

(sp)

ν

Tµν

 

Tµν

(ksrpl)

µ

 

 

 

 

p=l

 

 

 

 

 

 

 

 

 

 

 

 

and as usually, el = [al,ν , bl,ν ]T. Further, using the T -matrix equation sl = T lel, we obtain

 

 

 

 

 

 

 

N

 

 

 

 

 

 

 

[(sl)

 

] = [(Tl)

 

]

 

11

 

 

31

(ksrpl)

 

 

, (2.146)

ν

νν

 

(ksr0l) [eµ] +

Tµν

(sp)

µ

 

 

 

 

Tµν

 

 

 

 

 

p=l

and since (cf. (B.74) and (B.75))

Tν31µ (ksrlp) = Tµν31 (ksrpl)

and

 

 

 

Tν11µ (−ksr0l) = Tν11µ (ksr

we see that (2.144) and (2.146) coincide. The scattered field is a superposition

individual particles,

l0) = Tµν11 (ksr0l) ,

of fields that are scattered from the

N

Es(r) = Es,l (rl)

l=1

N

 

= fl,µM µ3 (ksrl) + gl,µN µ3 (ksrl) ,

(2.147)

l=1 µ

 

whence, using the addition theorem


136 2 Null-Field Method

M µ3 (ksrl)

= 33

(

 

ksr0l) M ν3 (ksr)

for

r > r0l ,

N µ3 (ksrl)

Tµν

 

 

N ν3 (ksr)

 

 

 

we derive the scattered-field expansion centered at O

 

Es(r) = fν M ν3 (ksr) + gν N ν3 (ksr)

 

 

ν

 

 

 

 

 

 

 

 

with

 

N

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

 

33

( ksr0l)

 

(2.148)

 

[sν ] =

 

 

Tµν

(sl)

µ

.

 

 

 

 

 

 

 

 

l=1

Since,

Tνµ11 (ksr0l) = Tµν11 (−ksr0l) = Tµν33 (−ksr0l) ,

we see that (2.145) and (2.148) are identical.

2.6.4 Formulation with Phase Shift Terms

For an ensemble of N particles with αl = βl = γl = 0, l = 1, 2, . . . , N, the system T -matrix is given by

N N

 

T = T 11 (ksr0l) AlpT pT 11 (−ksr0p) .

(2.149)

l=1 p=1

In (2.149), the translation matrices T 11(−ksr0p) and T 11(ksr0l) give the relations between the expansion coe cients of the incident and scattered fields in di erent coordinate systems. In the present analysis, these relations are derived by using the direct phase di erences between the electromagnetic fields in di erent coordinate systems.

For a vector plane wave of unit amplitude and wave vector ke, ke = ksek , we have

Ee (rl) = epolejksek ·r0l ejksek ·(r−r0l )

= ejksek ·r0l aν M 1ν (ksrl) + bν N 1ν (ksrl)

ν

=al,ν M 1ν (ksrl) + bl,ν N 1ν (ksrl)

ν

and therefore

al,ν

 

aν

 

bl,ν

= ejksek ·r0l

bν

.

 

 

Further, using the far-field representation of the field scattered by the lth particle,


 

 

 

 

 

 

 

 

 

 

 

 

2.6 Multiple Particles 137

E

 

(r

) =

ejksrl

!E

 

(e ) + O

1

"

 

 

rl

s∞,l

 

 

 

s,l

l

 

 

 

 

r

 

 

rl

and the approximation

 

 

 

 

 

 

 

 

 

 

 

 

ejksrl

=

ejksr ejkser ·r0l

1 + O

 

1

,

 

 

 

 

 

 

 

 

 

rl

 

 

 

 

r

 

 

 

r

we see that the angular-dependent vector of scattering coe cients

N

s (er ) = ejkser ·r0l sl

l=1

approximates the s vector in the far-field region, and that the angulardependent transition matrix

N N

 

T (er ) = ejks(ek ·r0p −er ·r0l )AlpT p

(2.150)

l=1 p=1

approximates the T matrix in the far-field region. For spherical particles, this method is known as the generalized multiparticle Mie-solution [272, 273].

Equation (2.150) shows that we have to impose

dim (T ) = dim AlpT p = dim (T lp) ,

where T lp = AlpT p. Assuming dim(T ) = 2Nmax × 2Nmax, we can set Nmax(p) = Nmax for all p = 1, 2, . . . , N, and in this case, dim(T ) = dim(T p).

Alternatively, we can set Nmax

= maxp Nmax(p)

and use the convention

(T

)

0 whenever ν > 2N

 

 

(l) and µ > 2Nmax(p). This formulation

 

lp νµ

 

max

 

11

avoids the computation of the translation matrices T11 and involves only the

inversion of the global matrix A. The dimensions of T

depend on translation

distances and are proportional to the overall dimension of the cluster, while the dimension of A is determined by the size parameters of the individual particles. Therefore, the generalized multiparticle Mie-solution is limited by the largest possible individual particle size in a cluster and not by the overall cluster size. However, the angular-dependent transition matrix can not be used in the analytical orientation-averaging procedure described in Sect. 1.5 and in view of our computer implementation, this method is not e ective for T -matrix calculations.

2.6.5 Recursive Aggregate T -matrix Algorithm

If the number of particles increases, the dimension of the global matrix A becomes excessively large. Wang and Chew [250, 251] proposed a recursive T - matrix algorithm, which computes the T matrix of a system of n components by using the transition matrices of the newly added q components and the


,Ncs p=1

138 2 Null-Field Method

T matrix of the previous system of n − q components. In this section we use the recursive T -matrix algorithm to analyze electromagnetic scattering by a system of identical particles randomly distributed inside an “imaginary” spherical surface.

Let us consider Ncs circumscribing spheres with radii Rcs(k), k = 1, 2, . . . , Ncs, in increasing order. Inside the sphere of radius Rcs(1) there are N(1) particles having their centers located at r(1)0l , l = 1, 2, . . . , N(1), and in each spherical shell bounded by the radii Rcs(k − 1) and Rcs(k) there are N(k) particles having their centers located at r(0kl ), l = 1, 2, . . . , N(k). Obviously, N = N(p) is the total number of particles and Rcs(Ncs) is the radius of the circumscribing sphere containing the particles. For simplicity, we assume that the particles are identical and have the same spatial orientation. The scattering geometry for the problem under examination is depicted in Fig. 2.7.

At the first iteration step, we compute the system T -matrix T (1) of all particles situated inside the sphere of radius Rcs(1). At the iteration step k, we compute the system T -matrix T (k) of all particles situated inside the sphere of radius Rcs(k) by considering a [N(k) + 1]-scatterer problem. In fact, the transition matrix T (k) is computed by using the system T -matrix T (k−1) of the previous ,kp=11 N(p) particles situated inside the sphere of radius Rcs(k − 1) and the individual transition matrix T p of all N(k) particles situated in the spherical shell between Rcs(k − 1) and Rcs(k). In this specific case, the blockmatrix components of the global matrix A are given by

All

= I ,

l = 1, 2, . . . , N(k) + 1 ,

 

 

 

 

 

 

Alp = −T pT 31

 

 

 

l = p ,

l, p = 1, 2, . . . , N(k) ,

 

 

ksrlp(k)

,

 

 

Al,N(k)+1

=

T

pT

31

k

r(k)

=

T

pT

31

 

k

r(k)

, l = 1, 2, . . . ,

N

(k) ,

 

 

 

 

s

l0

 

 

 

 

s

0l

 

 

AN(k)+1,l = −T (k−1)T 31 ksr(0kl ) , l = 1, 2, . . . , N(k) .

Rcs(1)

Rcs(k-1)

 

 

 

O

rol

(k)

 

O

 

 

 

 

Rcs(Ncs)

R

(k)

 

 

 

cs

Fig. 2.7. Illustration of the recursive T -matrix algorithm for many spheres